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This list of "Top 100 Anime Series Of All Time" will feature what I consider to be the 100 greatest anime series ever made. Some of the qualifying factors taken into consideration for a series being deemed great are, entertainment value, popularity, lasting appeal, quality of writing, originality and significance to the medium of anime. I didn't take just one factor into consideration. I took many as you can see by my description, this is not a list for most popular anime only.
IMDb: Most Popular Animation Titles